Prepare the slaw: Combine the cabbage, carrots, scallions, and cilantro in a medium bowl. Whisk together the rice vinegar, sesame oil, soy sauce, honey, and a pinch of salt, then toss with the vegetables until evenly coated.
Make the wonton chips: Add neutral oil to a small skillet. Slice wonton wrappers into 1/2 inch strips. When oil is hot, add strips. Cook for about 1-2 min or until the chips brown. It should happen pretty quickly. Transfer to a paper towel lined plate while you cook the tuna.
Sear the tuna: Pat the tuna dry and brush all sides with soy sauce. Add sesame to a plate in an even layer. Coat all sides of the tune with the seeds. Heat the neutral oil in a cast-iron skillet over high heat until just smoking. Sear the tuna for about 30–45 seconds per side, leaving the center rare. Transfer to a cutting board and let rest for a minute before slicing thinly against the grain.
Toast the brioche: Toast the brioche until golden and crisp.
Assemble the sandwiches: Spread a generous layer of spicy mayo on each slice of brioche. Arrange the sliced seared tuna followed by a generous pile of sesame slaw. Top with crispy wonton strips. Finish with the remaining brioche bun. Slice and enjoy!